Well I gave that a try and did not have good results. Now I didn't have a bunch of time to fiddle with things but it just did not work.
I set the timings like you said and it would get past POST but would lock up as it was getting into Vista. With regards to the sync setting, I didn't really go for that as if I set it to that it would set the memory at 586Mhz, so I'm not sure how that would achieve better performance.
Anyways, I set the timings and tried it at a 3:2 ratio what gave me 938Mhz(?, about that forgot exactly). Now that did not get into Vista as I mentioned, so I set the speed back down to 879MHz and tried again. Again it would not get into Vista, at that point I just set all of the timings back to auto, except for the tCL, tRCD, tRP, and tRAS. After that it went back into Vista.
So I'm thinking that it is most likely not your timings, but my board. This P5N-E SLI board just doesn't seem to like anything with memory and even quad cores can't OC very well on it. I'm thinking I might just have to leave it the way it is until I can get a new motherboard.
I will try to play with it all again as soon as I have time, maybe tonight, and will let you know if I get anywhere.