Honestly, if you're worried about Crysis, item#1 is going to be your GPU. Unless you're packing a beast of a GPU (or two), your CPU isn't going to be what slows you down right now.
2.0 V is fine for your memory, as long as you have some airflow over them. Keep the timings loose until you're done overclocking the CPU, but the memory is rated for what you're trying to do, so it shouldn't be an issue. 4-4-4-12 timings will be a bit of a toss-up with your memory, you'll almost certainly need 2.0-2.1 V to do it. Mine's rated like yours, and I managed it. But other sticks don't - luck of the draw, really.
Case pics would be nice.
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